Copper/ruthenium relay catalysis for stereodivergent construction of 1,4-nonadjacent stereocenters: mechanistic investigation using DFT calculations-Reference-Cited by-同舟云学术

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Copper/ruthenium relay catalysis for stereodivergent construction of 1,4-nonadjacent stereocenters: mechanistic investigation using DFT calculations

Published:2024 Issue:15 Volume:11 Page:4231-4248
ISSN:2052-4129
Container-title:Organic Chemistry Frontiers
language:en
Short-container-title:Org. Chem. Front.

Author:

Huang Congcong¹,Yang Biyao¹,Zhang Keying¹,Li Juan¹^ORCID

Affiliation:

1. College of Chemistry and Materials Science, Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications, Jinan University, Guangzhou, Guangdong 510632, P. R. China

Abstract

DFT calculations were used to explore the detailed reaction mechanism, and the origins of stereodivergence, in the Cu/Ru dual-catalyzed hydroalkylation of racemic allylic alcohols and racemic ketimine esters.

Funder

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/QO/D4QO00780H

Reference144 articles.

1. D. A.Evans and J. S.Johnson , in Comprehensive Asymmetric Catalysis , ed. E. N. Jacobsen , A. Pfaltz and H. Yamamoto , Springer , New York , 1999 , vol. 3 , p. 1177

2. Comprehensive Chirality , ed. E. M. Carreira and H. Yamamoto , Elsevier Science , Amsterdam , 2012 , vol. 1

3. Dual Catalysis Becomes Diastereodivergent

4. Diastereodivergent Processes in Palladium-Catalyzed Allylic Alkylation

5. E. M.Carreira and L.Kvaerno , Classics in Stereoselective Synthesis , Wiley , Weinheim , 2009

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