High-performance p-type elemental Te thermoelectric materials enabled by the synergy of carrier tuning and phonon engineering

Author:

An Decheng1234ORCID,Chen Shaoping1234,Zhai Xin1234,Yu Yuan5678,Fan Wenhao9234,Zhang Tingting10234,Liu Yequn1112131415,Wu Yucheng1234,Wang Wenxian1234,Snyder G. Jeffrey16171819ORCID

Affiliation:

1. College of Materials Science and Engineering

2. Taiyuan University of Technology

3. Taiyuan 030024

4. P. R. China

5. I. Physikalisches Institut (IA)

6. RWTH Aachen University

7. 52074 Aachen

8. Germany

9. College of Physics and Optoelectronics

10. Institute of Advanced Forming and Intelligent Equipment

11. Analytical Instrumentation Center

12. State Key Laboratory of Coal Conversion

13. Institute of Coal Chemistry

14. Chinese Academy of Sciences

15. Taiyuan 030001

16. Department of Materials Science and Engineering

17. Northwestern University

18. Evanston

19. USA

Abstract

An outstanding figure-of-merit zT ≈ 1.06 at 600 K for p-type elemental Te thermoelectrics is realized by synergistically tuning their carrier and phonon transport behaviors via a multicomponent alloying strategy.

Funder

Shanxi Scholarship Council of China

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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