Chemical control of spin–lattice relaxation to discover a room temperature molecular qubit-Reference-Cited by-同舟云学术

Chemical control of spin–lattice relaxation to discover a room temperature molecular qubit

Published:2022 Issue:23 Volume:13 Page:7034-7045
ISSN:2041-6520
Container-title:Chemical Science
language:en
Short-container-title:Chem. Sci.

Author:

Amdur M. Jeremy¹,Mullin Kathleen R.²,Waters Michael J.²^ORCID,Puggioni Danilo²^ORCID,Wojnar Michael K.¹,Gu Mingqiang²,Sun Lei³^ORCID,Oyala Paul H.⁴^ORCID,Rondinelli James M.²^ORCID,Freedman Danna E.¹⁵^ORCID

Affiliation:

1. Department of Chemistry, Massachusetts Institute of Technology, Cambridge, Massachusetts, 02139, USA

2. Department of Materials Science and Engineering, Northwestern University, Evanston, Illinois, 60208, USA

3. Center for Nanoscale Materials, Argonne National Laboratory, Argonne, Illinois, 60439, USA

4. Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, California, 91125, USA

5. Department of Chemistry, Northwestern University, Evanston, Illinois, 60208, USA

Abstract

Elucidating the role of specific vibrational modes in spin lattice relaxation is a key step to designing room temperature qubits. We executed an experimental and theoretical study on a series of Cu2+ qubits to increase their operating temperature.

Funder

Dow Chemical Company

U.S. Department of Energy

National Science Foundation

Office of Science

Basic Energy Sciences

Argonne National Laboratory

Northwestern University

California Institute of Technology

Laboratory Directed Research and Development

Publisher

Royal Society of Chemistry (RSC)