High-coordination Fe–N4SP single-atom catalysts via the multi-shell synergistic effect for the enhanced oxygen reduction reaction of rechargeable Zn–air battery cathodes

Author:

Liu Jiaqi1,Chen Weibin2,Yuan Shuang134ORCID,Liu Tie5,Wang Qiang15ORCID

Affiliation:

1. School of Metallurgy, Northeastern University, Shenyang 110819, China

2. School of Materials Science and Engineering, Peking University, Beijing 100871, China

3. Key Laboratory of Ecological Metallurgy of Multimetallic Mineral (Ministry of Education), Northeastern University, Shenyang 110819, China

4. Engineering Research Center of Frontier Technologies for Low-carbon Steelmaking (Ministry of Education), Liaoning Low-carbon Steelmaking Technology Engineering Research Center, Shenyang 110819, China

5. Key Laboratory of Electromagnetic Processing of Materials (Ministry of Education), Northeastern University, Shenyang 110819, China

Abstract

Novel Fe single-atom catalysts with highly coordinated Fe–N4SP structures were designed via the multi-coordination-shell synergistic effect. The optimization of the catalysts enhances their ORR activity in alkaline/acidic media towards rechargeable Zn–air batteries.

Funder

Fundamental Research Funds for the Central Universities

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Nuclear Energy and Engineering,Renewable Energy, Sustainability and the Environment,Environmental Chemistry

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