The catalytic and radical mechanism for ethanol oxidation to acetic acid-Reference-Cited by-同舟云学术

The catalytic and radical mechanism for ethanol oxidation to acetic acid

Published:2019 Issue:79 Volume:55 Page:11833-11836
ISSN:1359-7345
Container-title:Chemical Communications
language:en
Short-container-title:Chem. Commun.

Author:

Mostrou Sotiria¹²³⁴⁵^ORCID,Nagl Andreas⁶⁷⁸⁹¹⁰,Ranocchiari Marco¹¹¹²¹³⁵^ORCID,Föttinger Karin⁶⁷⁸⁹¹⁰,van Bokhoven Jeroen A.¹²³⁴⁵^ORCID

Affiliation:

1. Institute for Chemical and Bioengineering

2. Department of Chemistry and Applied Biosciences

3. ETH Zurich

4. 8093 Zurich

5. Switzerland

6. Institute of Material Chemistry

7. Division Physical Chemistry

8. TU Wien

9. 1060 Wien

10. Austria

11. Laboratory for Catalysis and Sustainable Chemistry

12. Paul Scherrer Institute

13. 5232 Villigen

Abstract

Liquid-phase ethanol oxidation to acetic acid proceeds in two steps: catalytic ethanol oxidation and non-catalytic acetaldehyde autoxidation. The balance between the two-steps coincides in the acetic acid formation and provides information for designing selective catalysts.

Funder

Austrian Science Fund

Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,Metals and Alloys,Surfaces, Coatings and Films,General Chemistry,Ceramics and Composites,Electronic, Optical and Magnetic Materials,Catalysis

Link

http://pubs.rsc.org/en/content/articlepdf/2019/CC/C9CC05813C

Reference25 articles.

1. Recent advances in processes and catalysts for the production of acetic acid

2. Formation of Acetic Acid by Aqueous-Phase Oxidation of Ethanol with Air in the Presence of a Heterogeneous Gold Catalyst

3. Aerobic oxidation of aqueous ethanol using heterogeneous gold catalysts: Efficient routes to acetic acid and ethyl acetate

4. Catalytic oxidation of aqueous bioethanol: an efficient upgrade from batch to flow

5. C–C Cleavage by Au/TiO2 during Ethanol Oxidation: Understanding Bandgap Photoexcitation and Plasmonically Mediated Charge Transfer via Quantitative in Situ DRIFTS

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