Determination of the <sup>144</sup>Ce/<sup>238</sup>U atomic ratio in spent nuclear fuel using double spike isotope dilution mass spectrometry-Reference-Cited by-同舟云学术

Determination of the ¹⁴⁴Ce/²³⁸U atomic ratio in spent nuclear fuel using double spike isotope dilution mass spectrometry

Published:2022 Issue:6 Volume:37 Page:1288-1297
ISSN:0267-9477
Container-title:Journal of Analytical Atomic Spectrometry
language:en
Short-container-title:J. Anal. At. Spectrom.

Author:

Beaumais Aurélien¹^ORCID,Nonell Anthony¹,Caussignac Céline¹,Mialle Sébastien¹,Stadelmann Guillaume²,Janin Myriam³,Isnard Hélène¹,Aubert Michel¹,Vercouter Thomas⁴,Chartier Frédéric⁵

Affiliation:

1. DES – Service d'Etudes Analytiques et de Réactivité des Surfaces (SEARS), CEA, Université Paris-Saclay, F-91191 Gif Sur Yvette, France

2. IAEA laboratories, Friedenstrasse, 1, A-2444 Seibersdorf, Austria

3. Direction des Services Départementaux de l’Éducation nationale de Moselle, France

4. DES – Service d’Etudes des Matériaux Irradiés, CEA, Université Paris-Saclay, F-91191 Gif Sur Yvette, France

5. DES – Département de Physico-Chimie (DPC), CEA, Université Paris-Saclay, F-91191 Gif Sur Yvette, France

Abstract

Determination of the 144Ce/238U ratio in spent nuclear fuels using the double isotope dilution technique associated with thermal ionization mass spectrometry measurements.

Publisher

Royal Society of Chemistry (RSC)

Subject

Spectroscopy,Analytical Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2022/JA/D2JA00052K

Reference40 articles.

1. NEA/NSC/WPNCS , Spent Nuclear Fuel Assay Data for Isotopic Validation. State-Of-The-Art Report, N. Science , 2011 , OECD , Paris . pp. 1–97

2. M.-M.Bé , et al., Table of radionuclides (Vol. 8 - A = 41 to 198) , in Monographie BIPM-5, BIPM , Editor. 2016 , BIPM: Pavillon de Breteuil, F-92310 Sevres, France

3. Isotope dilution mass spectrometry: what can it contribute to accuracy in trace analysis?

4. Isotope dilution mass spectrometry (IDMS) of the elements

5. Determination of erbium in nuclear fuels by isotope dilution thermal ionization mass spectrometry and glow discharge mass spectrometry

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