Experimental and theoretical investigation of oxidative methane activation on Pd–Pt catalysts
Author:
Affiliation:
1. Key Laboratory of Advanced Manufacturing Technology for Automobile Parts
2. Ministry of Education
3. Chongqing University of Technology
4. Chongqing 400050
5. China
Abstract
Density functional theory and measurements of rate are used to provide evidence for the rate determining step and requirements of the active site for CH4 combustion on Pd–Pt bimetallic catalysts in five different distinct kinetic regimes.
Funder
National Natural Science Foundation of China
Publisher
Royal Society of Chemistry (RSC)
Subject
General Chemical Engineering,General Chemistry
Link
http://pubs.rsc.org/en/content/articlepdf/2019/RA/C9RA00735K
Reference34 articles.
1. Pathways and kinetics of methane and ethane C–H bond cleavage on PdO(101)
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3. First-Principles Investigation of C–H Bond Scission and Formation Reactions in Ethane, Ethene, and Ethyne Adsorbed on Ru(0001)
4. High Selectivity for Primary C–H Bond Cleavage of Propane σ-Complexes on the PdO(101) Surface
5. Characterisation and microstructure of Pd and bimetallic Pd–Pt catalysts during methane oxidation
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