Visible-light-induced aerobic oxidation of alcohols to aldehydes/ketones <i>via</i> solvated dispersion intermediates-Reference-Cited by-同舟云学术

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Visible-light-induced aerobic oxidation of alcohols to aldehydes/ketones via solvated dispersion intermediates

Published:2024 Issue:13 Volume:26 Page:7902-7910
ISSN:1463-9262
Container-title:Green Chemistry
language:en
Short-container-title:Green Chem.

Author:

Lei Wenlong¹²,Liu Runze³,Li Rengui¹²^ORCID,Liu Yan¹²^ORCID,Li Can¹²^ORCID

Affiliation:

1. State Key Laboratory of Catalysis, Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, China

2. University of Chinese Academy of Sciences, Beijing, China

3. Institute of Molecular Sciences and Engineering, Institute of Frontier and Interdisciplinary Science, Shandong University, Qingdao, China

Abstract

Visible-light-induced fast and selective aerobic oxidation of alcohols to aldehydes/ketones with HBr as a mediator in ethyl acetate enables high selectivity (up to 99%) and high conversion (up to 97%) for a broad range of alcohols.

Funder

National Natural Science Foundation of China

Postdoctoral Research Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/GC/D4GC01210K

Reference55 articles.

1. J. E.Bäckvall , Modern Oxidation Methods , Wiley-VCH , 2004

2. Green, Catalytic Oxidations of Alcohols

3. Oxidation of Alcohols with Molecular Oxygen on Solid Catalysts

4. A “universal” catalyst for aerobic oxidations to synthesize (hetero)aromatic aldehydes, ketones, esters, acids, nitriles, and amides

5. Pyridinium chlorochromate. An efficient reagent for oxidation of primary and secondary alcohols to carbonyl compounds

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