Competitive pathways of methane activation on Zn2+-modified ZSM-5 zeolite: H/D hydrogen exchange with Brønsted acid sites versus dissociative adsorption to form Zn-methyl species-Reference-Cited by-同舟云学术

Competitive pathways of methane activation on Zn2+-modified ZSM-5 zeolite: H/D hydrogen exchange with Brønsted acid sites versus dissociative adsorption to form Zn-methyl species

Published:2016 Issue:16 Volume:6 Page:6381-6388
ISSN:2044-4753
Container-title:Catalysis Science & Technology
language:en
Short-container-title:Catal. Sci. Technol.

Author:

Arzumanov Sergei S.¹²³⁴⁵,Gabrienko Anton A.¹²³⁴⁵,Freude Dieter⁶⁷⁸⁹,Stepanov Alexander G.¹²³⁴⁵

Affiliation:

1. Boreskov Institute of Catalysis

2. Siberian Branch of the Russian Academy of Sciences

3. Novosibirsk 630090

4. Russia

5. Department of Natural Sciences

6. Fakultät für Physik und Geowissenschaften

7. Universität Leipzig

8. 04103 Leipzig

9. Germany

Abstract

Zn-methyl species is not responsible for facilitation of the H/D hydrogen exchange reaction of methane with Brønsted acid sites of Zn²⁺/H-ZSM-5 zeolite.

Funder

Deutsche Forschungsgemeinschaft

Publisher

Royal Society of Chemistry (RSC)

Subject

Catalysis

Link

http://pubs.rsc.org/en/content/articlepdf/2016/CY/C6CY00878J

Reference45 articles.

1. Structure and Density of Active Zn Species in Zn/H-ZSM5 Propane Aromatization Catalysts

2. Selective ethane conversion into aromatic hydrocarbons over Zn-ZSM-11 zeolite

3. Methane transformation into aromatic hydrocarbons by activation with ethane over Zn-ZSM-11 zeolite

4. Improvement of methane activation using n-hexane as co-reactant over Zn/HZSM-11 zeolite

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