Electron paramagnetic resonance spectroscopic studies of the electron transfer reaction of Hantzsch ester and a pyrylium salt-Reference-Cited by-同舟云学术

Electron paramagnetic resonance spectroscopic studies of the electron transfer reaction of Hantzsch ester and a pyrylium salt

Published:2018 Issue:52 Volume:8 Page:29924-29927
ISSN:2046-2069
Container-title:RSC Advances
language:en
Short-container-title:RSC Adv.

Author:

Sebők-Nagy K.¹²³⁴⁵,Rózsár D.⁶⁴⁵,Puskás L. G.⁶⁴⁵,Balázs Á.⁶⁴⁵^ORCID,Páli T.¹²³⁴⁵^ORCID

Affiliation:

1. Institute of Biophysics

2. Biological Research Centre

3. Hungarian Academy of Sciences

4. H-6726 Szeged

5. Hungary

6. AVICOR Ltd.

Abstract

The oxidation of Hantzsch ester by a pyrylium cation takes 3 place via electron–proton–electron transfer. The present in-depth EPR study of the radical reactions of a NADH analogue indicate a complex electron transfer mechanism in the title reaction.

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemical Engineering,General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2018/RA/C8RA05693E

Reference33 articles.

1. Which Hydrogen Atom Is First Transferred in the NAD(P)H Model Hantzsch Ester Mediated Reactions via One-Step and Multistep Hydride Transfer?

2. Kinetic and mechanistic investigation on the oxidation of Hantzsch 1,4-dihydropyridines with the tropylium cation: a model for NADH oxidation

3. Kinetic, thermodynamic and mechanistic studies on the reduction of carbenium ions by NAD(P)H analogues

4. Determination of the C4H Bond Dissociation Energies of NADH Models and Their Radical Cations in Acetonitrile

5. 1-Benzyldihydronicotinamide—A Model for Reduced DPN

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