WO3 nanosheets rich in oxygen vacancies for enhanced electrocatalytic N2 reduction to NH3-Reference-Cited by-同舟云学术

WO3 nanosheets rich in oxygen vacancies for enhanced electrocatalytic N2 reduction to NH3

Published:2019 Issue:41 Volume:11 Page:19274-19277
ISSN:2040-3364
Container-title:Nanoscale
language:en
Short-container-title:Nanoscale

Author:

Kong Wenhan¹²³⁴⁵,Zhang Rong⁶⁷⁸⁵,Zhang Xiaoxue⁹¹⁰¹¹¹²⁵,Ji Lei⁶⁷⁸⁵,Yu Guangsen⁶⁷⁸⁵,Wang Ting⁹¹⁰¹¹¹²⁵^ORCID,Luo Yonglan⁹¹⁰¹¹¹²⁵^ORCID,Shi Xifeng¹³¹⁴¹⁵¹⁶⁵,Xu Yuanhong¹²³⁴⁵^ORCID,Sun Xuping⁶⁷⁸⁵^ORCID

Affiliation:

1. College of Materials Science and Engineering

2. College of Life Sciences

3. Qingdao University

4. Qingdao 266071

5. China

6. Institute of Fundamental and Frontier Sciences

7. University of Electronic Science and Technology of China

8. Chengdu 610054

9. Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province

10. College of Chemistry and Chemical Engineering

11. China West Normal University

12. Nanchong 637002

13. College of Chemistry

14. Chemical Engineering and Materials Science

15. Shandong Normal University

16. Jinan 250014

Abstract

WO₃ nanosheets rich in oxygen vacancies are efficient for electrocatalytic N₂-to-NH₃ fixation under ambient conditions with a NH₃ yield of 17.28 μg h⁻¹ mg_cat.⁻¹ and a faradaic efficiency of 7.0% in 0.1 M HCl.

Funder

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science

Link

http://pubs.rsc.org/en/content/articlepdf/2019/NR/C9NR03678D

Reference56 articles.

1. Nitrogen Cycle Electrocatalysis

2. Catalytic Synthesis of Ammonia—A “Never-Ending Story”?

3. How a century of ammonia synthesis changed the world

4. T. Vegge , R. Z.Sørensen , A.Klerke , J. S.Hummelshøj , T.Johannessen , J. K.Nørskov and C. H.Christensen , Indirect Hydrogen Storage in Metal Ammines , British Welding Research Association , 2008 , pp. 533–564

5. Transformation of Coordinated Dinitrogen by Reaction with Dihydrogen and Primary Silanes

Cited by 89 articles. 订阅此论文施引文献订阅此论文施引文献，注册后可以免费订阅5篇论文的施引文献，订阅后可以查看论文全部施引文献

1. A comprehensive review on electrochemical green ammonia synthesis: From conventional to distinctive strategies for efficient nitrogen fixation;Applied Energy;2023-12

2. Rebalancing Hydrogenation and Dehydration Performances for Efficient Hydrodeoxygenation of Biomass Derivatives to Match Reaction Temperature-Induced Rate-Determining Step Switch;Industrial & Engineering Chemistry Research;2023-10-23

3. Efficient electrocatalytic conversion of N2 to NH3 using oxygen-rich vacancy lithium niobate cubes;Chinese Journal of Chemical Engineering;2023-10

4. Two-Dimensional Metal–Organic Framework TM Catalysts for Electrocatalytic N2 and CO2 Reduction: A Density Functional Theory Investigation;Crystals;2023-09-26

5. A comparative study of RuO2 and Ru reveals the role of oxygen vacancies in electrocatalytic nitrogen reduction to ammonia under ambient conditions;Applied Catalysis A: General;2023-09