Untangling the intertwined: metallic to semiconducting phase transition of colloidal MoS2 nanoplatelets and nanosheets

Author:

Niebur André12ORCID,Söll Aljoscha1ORCID,Haizmann Philipp3,Strolka Onno123ORCID,Rudolph Dominik12ORCID,Tran Kevin45ORCID,Renz Franz45ORCID,Frauendorf André Philipp6ORCID,Hübner Jens56ORCID,Peisert Heiko3ORCID,Scheele Marcus3ORCID,Lauth Jannika1235ORCID

Affiliation:

1. Institute of Physical Chemistry and Electrochemistry, Leibniz University Hannover, Callinstr. 3a, D-30167 Hannover, Germany

2. Cluster of Excellence PhoenixD (Photonics, Optics, and Engineering – Innovation Across Disciplines), Hannover, Germany

3. Institute of Physical and Theoretical Chemistry, University of Tübingen, Auf der Morgenstelle 18, D-72076 Tübingen, Germany

4. Institute of Inorganic Chemistry, Leibniz University Hannover, Callinstr. 9, D-30167 Hannover, Germany

5. Laboratory of Nano and Quantum Engineering (LNQE), Leibniz University Hannover, Schneiderberg 39, D-30167 Hannover, Germany

6. Institute of Solid State Physics, Leibniz University Hannover, Appelstr. 2, D-30167 Hannover, Germany

Abstract

Colloidal ultrathin 2D MoS2 nanoplatelets and nanosheets provide a toolbox for future spin- and valleytronic applications. Colloidal chemistry offers innovative strategies to tune the materials' optoelectronic properties from metallic to semiconducting.

Funder

Gottfried Wilhelm Leibniz Universität Hannover

Deutsche Forschungsgemeinschaft

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science

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