Transmutation effects on long-term Cs retention in phyllosilicate minerals from first principles
Author:
Affiliation:
1. Physical Sciences Division
2. Pacific Northwest National Laboratory
3. Richland
4. USA
5. CCSE
6. Japan Atomic Energy Agency
7. Japan
Abstract
Thermodynamic analysis indicates that radiocesium transmutation in phyllosilicate mineral interlayers weakens the binding of remaining Cs and favors its desorption.
Funder
Japan Atomic Energy Agency
Publisher
Royal Society of Chemistry (RSC)
Subject
Physical and Theoretical Chemistry,General Physics and Astronomy
Link
http://pubs.rsc.org/en/content/articlepdf/2017/CP/C7CP04496H
Reference48 articles.
1. Selective Sorption and Fixation of Cations by Clay Minerals: A Review
2. Preferential adsorption of 137Cs to micaceous minerals in contaminated freshwater sediment
3. Reversible ion-exchange fixation of cesium-137 leading to mobilization from reservoir sediments
4. Quantitative analysis of radiocaesium retention in soils
5. Adsorption of cesium on minerals: A review
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1. Radiocesium interaction with clay minerals: Theory and simulation advances Post–Fukushima;Journal of Environmental Radioactivity;2019-12
2. Intensive evaluation of radiation stability of phlogopite single crystals under high doses of γ-ray irradiation;RSC Advances;2019
3. Radiocesium interaction with clay minerals: Theory and simulation advances Post–Fukushima;Journal of Environmental Radioactivity;2018-09
4. Reply to ''Comments on Radiation-damage Resistance In Phyllosilicate Minerals from First Principles and Implications For Radiocesium and Strontium Retention in Soils'';Clays and Clay Minerals;2017-10-01
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