Crystal reconstruction and defect healing enabled high-quality Sb2Se3 films for solar cell applications

Author:

Zhao Qi1,Che Bo1,Wang Haolin1,Peng Xiaoqi1,Yang Junjie1,Tang Rongfeng1ORCID,Zhu Changfei1,Chen Tao1ORCID

Affiliation:

1. Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, Department of Materials Science and Engineering, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei, 230026, China

Abstract

A post-sulfurization technique has been developed to refine Sb2Se3 crystallization. This process enables high-quality Sb2Se3 with a smooth surface, large compact crystal grains and benign [hkl] growth orientation. It also mitigates the device VOC deficit, owing to the healed deep level defects.

Funder

Institute of Energy, Hefei Comprehensive National Science Center

National Natural Science Foundation of China

National Key Research and Development Program of China

Fundamental Research Funds for the Central Universities

Chinese Academy of Sciences

Publisher

Royal Society of Chemistry (RSC)

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