Photoelectrochemical water splitting by hematite boosted in a heterojunction with B-doped g-C3N4 nanosheets and carbon nanotubes

Author:

Khan Irfan1ORCID,Benkó Tímea1,Horváth Anita1,Shen Shaohua2ORCID,Su Jinzhan2ORCID,Wang Yiqing2,Horváth Zsolt E.3,Németh Miklós1,Czigány Zsolt3ORCID,Zámbó Dániel3,Pap József Sándor1

Affiliation:

1. Department of Surface Chemistry and Catalysis, HUN-REN Centre for Energy Research, Konkoly-ThegeM. Street 29-33, Budapest, 1121, Hungary

2. International Research Center for Renewable Energy (IRCRE), State Key Laboratory of Multiphase Flow in Power Engineering (MFPE), Xi'an Jiaotong University, Xi'an, China

3. HUN-REN Centre for Energy Research, Institute of Technical Physics and Materials Science, Konkoly-Thege M. Street 29-33, Budapest, 1121, Hungary

Abstract

Enhanced PEC water splitting with an α-Fe2O3/B-C3N4 type II heterojunction. Use of pyrolytic (p-)CNT to improve photoanodic current density. Improved electrical conductivity for facile charge separation & transfer. DFT hints at a Z-scheme mechanism.

Funder

National Research, Development and Innovation Office

Publisher

Royal Society of Chemistry (RSC)

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