Dynamic disorder, phonon lifetimes, and the assignment of modes to the vibrational spectra of methylammonium lead halide perovskites

Author:

Leguy Aurélien M. A.123,Goñi Alejandro R.45678,Frost Jarvist M.9103,Skelton Jonathan9103,Brivio Federico9103,Rodríguez-Martínez Xabier4567,Weber Oliver J.9103,Pallipurath Anuradha111213,Alonso M. Isabel4567,Campoy-Quiles Mariano4567,Weller Mark T.9103,Nelson Jenny1231415,Walsh Aron9103,Barnes Piers R. F.8167

Affiliation:

1. Physics department

2. Imperial College London

3. UK

4. Institut de Ciència de Materials de Barcelona (ICMAB-CSIC)

5. Campus UAB

6. 08193 Bellaterra

7. Spain

8. ICREA

9. Chemistry department

10. University of Bath

11. School of chemistry

12. National University of Ireland Galway

13. Ireland

14. SPECIFIC

15. College of Engineering

16. 08010 Barcelona

Abstract

Raman and THz spectra of CH3NH3PbX3 interpreted with a catalogue of computed vibrations and their influence on heat and electrical transport.

Funder

Royal Irish Academy

European Research Council

Engineering and Physical Sciences Research Council

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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