On the origin of reactivity variation upon sequential ligation: the [Re(Cl)x]+/CH4 (x = 1

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On the origin of reactivity variation upon sequential ligation: the [Re(Cl)x]+/CH4 (x = 1–3) couples

Published:2021 Issue:42 Volume:23 Page:24319-24327
ISSN:1463-9076
Container-title:Physical Chemistry Chemical Physics
language:en
Short-container-title:Phys. Chem. Chem. Phys.

Author:

Yan Linghui¹²,Li Shihan¹²,Zhou Shaodong¹²^ORCID

Affiliation:

1. College of Chemical and Biological Engineering, Zhejiang Provincial Key Laboratory of Advanced Chemical Engineering Manufacture Technology, Zhejiang University, 310027 Hangzhou, P. R. China

2. Institute of Zhejiang University – Quzhou, 78 Jiuhua Boulevard North, 324000 Quzhou, P. R. China

Abstract

The reactivity of the clusters decreases in turn as the number of chlorine ligands increases!

Funder

National Natural Science Foundation of China

Deutsche Forschungsgemeinschaft

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

Link

http://pubs.rsc.org/en/content/articlepdf/2021/CP/D1CP03468E

Reference69 articles.

1. Homogeneous Functionalization of Methane

2. Methane as raw material in synthetic chemistry: the final frontier

3. C–H activation

4. Intrinsic Reactivity of Diatomic 3d Transition-Metal Carbides in the Thermal Activation of Methane: Striking Electronic Structure Effects

5. Methane Activation by Gas Phase Atomic Clusters

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