Tunable product selectivity on demand: a mechanism-guided Lewis acid co-catalyst for CO<sub>2</sub> electroreduction to ethylene glycol-Reference-Cited by-同舟云学术

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Tunable product selectivity on demand: a mechanism-guided Lewis acid co-catalyst for CO₂ electroreduction to ethylene glycol

Published:2024 Issue:3 Volume:2 Page:823-833
ISSN:2753-801X
Container-title:EES Catalysis
language:en
Short-container-title:EES. Catal.

Author:

Li Yifei¹^ORCID,Calvinho Karin U. D.¹²^ORCID,Dhiman Mahak¹^ORCID,Laursen Anders B.¹²,Gu Hengfei¹,Santorelli Dominick¹,Clifford Zachary¹,Dismukes G. Charles¹³^ORCID

Affiliation:

1. Department of Chemistry and Chemical Biology, 123 Bevier Rd, Piscataway, NJ 08854, USA

2. RenewCO2 Inc., 418 Orchard Street, Cranford, NJ 07016-1745, USA

3. Waksman Institute of Technology, 190 Frelinghuysen Rd, Piscataway, NJ, USA

Abstract

This work illustrates the feasibility of using Lewis acid/base co-catalysts to change the established chemical reaction mechanism of an electrocatalyst to form a new, chemically predictable, more valuable product in high yield.

Funder

Small Business Innovation Research and Small Business Technology Transfer

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/EY/D3EY00237C

Reference43 articles.

1. Selective CO2 reduction to C3 and C4 oxyhydrocarbons on nickel phosphides at overpotentials as low as 10 mV

2. What would it take for renewably powered electrosynthesis to displace petrochemical processes?

3. Catalyst design strategies for stable electrochemical CO2 reduction reaction

4. Electrolytic CO2 Reduction in a Flow Cell

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