Dynamics over a Cu–graphite electrode during the gas-phase CO2 reduction investigated by APXPS

Author:

Arrigo Rosa12ORCID,Blume Raoul34,Large Alexander Ian2ORCID,Velasco-Vélez Juan Jesus34ORCID,Hävecker Michael34ORCID,Knop-Gericke Axel34,Held Georg2ORCID

Affiliation:

1. University of Salford, School of Science, Engineering and Environment, Cockcroft Building, Greater Manchester M5 4WT, UK

2. Diamond Light Source Ltd, Harwell Science & Innovation Campus, Didcot, Oxfordshire OX11 0DE, UK

3. Department of Inorganic Chemistry, Fritz-Haber-Institut der Max-Planck Gesellschaft, Faradayweg 4-6, 14195 Berlin, Germany

4. Max-Planck-Institut für Chemische Energiekonversion, Stiftstrasse 34-36, 45470 Mülheim an der Ruhr, Germany

Abstract

We use ambient pressure X-ray photoelectron and absorption spectroscopies coupled with on-line gas detection to investigate in situ performance and interface chemistry of an electrodeposited Cu on a carbon support under conditions of CO2 reduction.

Funder

Engineering and Physical Sciences Research Council

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry

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