Modification of an oxyhalide solid-solution photocatalyst with an efficient O2-evolving cocatalyst and electron mediator for two-step photoexcitation overall water splitting

Author:

Sun Wenzheng12ORCID,Luo Ying12,Xu Jun12,Guo Qiaoqi12,Deng Lidan3,Wang Zheng12ORCID,He Hong12ORCID

Affiliation:

1. State Key Joint Laboratory of Environment Simulation and Pollution Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China

2. University of Chinese Academy of Sciences, Beijing 100049, China

3. School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, China

Abstract

The decoration of high-crystallinity Bi4TaO8Cl0.9Br0.1 solid solution with CoOx cocatalyst and reduced graphene oxide promoted O2 generation and electron transfer, thus boosting active two-step excitation water splitting under visible light.

Funder

National Natural Science Foundation of China

China Postdoctoral Science Foundation

Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science

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