Diffusion equation for the longitudinal spectral diffusion: the case of the RIDME experiment-Reference-Cited by-同舟云学术

Diffusion equation for the longitudinal spectral diffusion: the case of the RIDME experiment

Published:2022 Issue:38 Volume:24 Page:23517-23531
ISSN:1463-9076
Container-title:Physical Chemistry Chemical Physics
language:en
Short-container-title:Phys. Chem. Chem. Phys.

Author:

Kuzin Sergei¹^ORCID,Jeschke Gunnar¹^ORCID,Yulikov Maxim¹^ORCID

Affiliation:

1. ETH Zürich, Department of Chemistry and Applied Bioscience, Laboratory of Physical Chemistry, Vladimir-Prelog-Weg 2, 8093 Zürich, Switzerland

Abstract

Relaxation-induced dipolar modulation enhancement (RIDME) time traces follow linear scaling law with proton concentration in homogeneous glassy water–glycerol samples and can be described quantitatively by a newly derived diffusion equation.

Funder

Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

Link

http://pubs.rsc.org/en/content/articlepdf/2022/CP/D2CP03039J

Reference41 articles.

1. Electron dipole–dipole interaction in ESEEM of nitroxide biradicals

2. A pulsed EPR method to determine distances between paramagnetic centers with strong spectral anisotropy and radicals: The dead-time free RIDME sequence

3. RIDME Spectroscopy with Gd(III) Centers

4. A. V.Astashkin , Mapping the structure of metalloproteins with RIDME , in Electron Paramagnetic Resonance Investigations of Biological Systems by Using Spin Labels, Spin Probes, and Intrinsic Metal Ions, Part A, of Methods in Enzymology , ed. P. Z. Qin and K. Warncke , Academic Press , 2015 , vol. 563, pp. 251–284

5. Comparison of PELDOR and RIDME for Distance Measurements between Nitroxides and Low-Spin Fe(III) Ions

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