Tandem electrocatalytic aziridination – ring expansion of simple aromatic olefins using ammonia and carbon dioxide-Reference-Cited by-同舟云学术

Tandem electrocatalytic aziridination – ring expansion of simple aromatic olefins using ammonia and carbon dioxide

Published:2023 Issue:3 Volume:25 Page:978-985
ISSN:1463-9262
Container-title:Green Chemistry
language:en
Short-container-title:Green Chem.

Author:

Vanhoof Jef R.¹^ORCID,Dirix Robin¹,De Vos Dirk E.¹^ORCID

Affiliation:

1. Centre For Membrane Separations, Adsorption, Catalysis and Spectroscopy for Sustainable Solutions (cMACS), KU Leuven, Celestijnenlaan 200F p.o. box 2454, 3001 Leuven, Belgium

Abstract

The telescoped electrochemical coupling of NH3 and CO2 with simple aromatic olefins is described, forming valuable N-heterocycles in an atom-efficient manner with overall yields of up to 91%. The same iodide catalyst is required for both steps.

Funder

Fonds Wetenschappelijk Onderzoek

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Environmental Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2023/GC/D2GC03879J

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