Conjugated polymers with controllable interfacial order and energetics enable tunable heterojunctions in organic and colloidal quantum dot photovoltaics

Author:

Zhong Yufei12ORCID,Kirmani Ahmad R.2ORCID,Lan Xinzheng3,Carpenter Joshua4,Rong-Hui Chew Annabel5,Awartani Omar46ORCID,Yu Liyang27ORCID,Niazi Muhammad R.2ORCID,Voznyy Oleksandr8ORCID,Hu Hanlin29,Ngongang Ndjawa Guy Olivier2,Tietze Max L.210,Salleo Alberto5,Ade Harald4,Sargent Edward H.8,Amassian Aram211ORCID

Affiliation:

1. School of Materials Science and Engineering (MSE), NingboTech University, No.1 South Qianhu Road, Ningbo, 315100, P. R. China

2. King Abdullah University of Science and Technology (KAUST), KAUST Solar Center (KSC), Physical Sciences and Engineering Division, Thuwal, 23955-6900, Saudi Arabia

3. School of Optical and Electronic Information and Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, Wuhan, Hubei, 430074, P. R. China

4. Department of Physics, Organic and Carbon Electronics Laboratories (ORaCEL), North Carolina State University, Raleigh, NC, 27695, USA

5. Department of Materials Science and Engineering, Stanford University, Stanford, CA, USA

6. Department of Mechanical Engineering, Maroun Semaan Faculty of Engineering and Architecture, American University of Beirut, Beirut, 1107-2020 Lebanon

7. School of Chemical Engineering, Sichuan University, Chengdu, 610064, P. R. China

8. Department of Electrical and Computer Engineering, University of Toronto, 10 King's College Road, Toronto, Ontario, M5S 3G4, Canada

9. Hoffman Institute of Advanced Materials, Shenzhen Polytechnic, 7098 Liuxian Boulevard, Shenzhen, 518055, P. R. China

10. Centre for Membrane Separations, Adsorption, Catalysis and Spectroscopy for Sustainable Solutions (cMACS), University of Leuven, Celestijnenlaan 200F box 2454, 3001, Leuven, Belgium

11. Department of Materials Science and Engineering, Organic and Carbon Electronic Laboratories (ORaCEL), North Carolina State University, Raleigh, NC, 27695, USA

Abstract

Top and bottom surfaces of polymer films are used to construct interfaces in heterojunction based devices, affecting device figure of merit significantly with their different aggregation states.

Funder

Natural Science Foundation of Zhejiang Province

Office of Naval Research

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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