Hemicubane topological analogs of the oxygen-evolving complex of photosystem II mediating water-assisted propylene carbonate oxidation-Reference-Cited by-同舟云学术

Hemicubane topological analogs of the oxygen-evolving complex of photosystem II mediating water-assisted propylene carbonate oxidation

Published:2022 Issue:15 Volume:58 Page:2532-2535
ISSN:1359-7345
Container-title:Chemical Communications
language:en
Short-container-title:Chem. Commun.

Author:

Koellner Connor A.¹,Gau Michael R.²,Polyak Aleksander¹,Bayana Manish¹,Zdilla Michael J.¹^ORCID

Affiliation:

1. Department of Chemistry, Temple University, 1901 N. 13th St., Philadelphia, PA, 19122, USA

2. Department of Chemistry, University of Pennsylvania, 231 S 34th St, Philadelphia, PA, 19104, USA

Abstract

A series of Ca–Mn hemicubane clusters with topological analogy to the biological oxygen evolving complex are prepared. Those with closest structural analogy are active in the electrochemical activation of water in the decomposition of propylene carbonate.

Funder

National Science Foundation

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,Metals and Alloys,Surfaces, Coatings and Films,General Chemistry,Ceramics and Composites,Electronic, Optical and Magnetic Materials,Catalysis

Link

http://pubs.rsc.org/en/content/articlepdf/2022/CC/D1CC05825H

Reference52 articles.

1. Recent developments in research on water oxidation by photosystem II

2. The O2-Evolving Complex of Photosystem II: Recent Insights from Quantum Mechanics/Molecular Mechanics (QM/MM), Extended X-ray Absorption Fine Structure (EXAFS), and Femtosecond X-ray Crystallography Data

3. Water-Splitting Chemistry of Photosystem II

4. Native structure of photosystem II at 1.95 Å resolution viewed by femtosecond X-ray pulses

5. Two Different Structures of the Oxygen-Evolving Complex in the Same Polypeptide Frameworks of Photosystem II

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