A rhodium-catalyzed C–H activation/cyclization approach toward the total syntheses of cassiarin C and 8-<i>O</i>-methylcassiarin A from a common intermediate-Reference-Cited by-同舟云学术

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A rhodium-catalyzed C–H activation/cyclization approach toward the total syntheses of cassiarin C and 8-O-methylcassiarin A from a common intermediate

Published:2024 Issue: Volume: Page:
ISSN:1477-0520
Container-title:Organic & Biomolecular Chemistry
language:en
Short-container-title:Org. Biomol. Chem.

Author:

Vargas Didier F.¹²^ORCID,Fonzo Santiago²^ORCID,Simonetti Sebastian O.¹²^ORCID,Kaufman Teodoro S.¹²^ORCID,Larghi Enrique L.¹²^ORCID

Affiliation:

1. Instituto de Química Rosario (IQUIR, CONICET-UNR), Universidad Nacional de Rosario, Suipacha 531, 2000, Rosario, Argentina

2. Facultad de Ciencias Bioquímicas y Farmacéuticas, Universidad Nacional de Rosario, Suipacha 531, 2000, Rosario, Argentina

Abstract

Cassiarin alkaloids were synthesized from a common intermediate, using a Rh-based C–H activation approach. DFT calculations shed light on an unusual H/D exchange.

Funder

Fondo para la Investigación Científica y Tecnológica

Alexander von Humboldt-Stiftung

Consejo Nacional de Investigaciones Científicas y Técnicas

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/OB/D4OB01122H

Reference138 articles.

1. In vitro antiplasmodial activity of 18 plants used in Congo Brazzaville traditional medicine

2. Ethnobotanical survey and in vitro antiplasmodial activity of plants used in traditional medicine in Burkina Faso

3. Diversity, Knowledge, and Use of Plants in Traditional Treatment of Diabetes in the Republic of Benin

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