PdP2 nanoparticles–reduced graphene oxide for electrocatalytic N2 conversion to NH3 under ambient conditions

Author:

Xie Hongtao12345ORCID,Geng Qin1234ORCID,Zhu Xiaojuan67894,Luo Yonglan67894ORCID,Chang Le1234ORCID,Niu Xiaobin1234ORCID,Shi Xifeng101112134,Asiri Abdullah M.1415161718ORCID,Gao Shuyan1920214ORCID,Wang Zhiming1234,Sun Xuping1234ORCID

Affiliation:

1. Institute of Fundamental and Frontier Sciences

2. University of Electronic Science and Technology of China

3. Chengdu 610054

4. China

5. College of Material Science and Engineering

6. Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province

7. College of Chemistry and Chemical Engineering

8. China West Normal University

9. Nanchong 637002

10. College of Chemistry

11. Chemical Engineering and Materials Science

12. Shandong Normal University

13. Jinan 250014

14. Chemistry Department

15. Faculty of Science & Center of Excellence for Advanced Materials Research

16. King Abdulaziz University

17. Jeddah 21589

18. Saudi Arabia

19. School of Chemistry and Chemical Engineering

20. Henan Normal University

21. Xinxiang 453007

Abstract

PdP2-reduced graphene oxide hybrid is efficient for ambient electrocatalytic N2-to-NH3 fixation with an NH3 yield rate of 30.3 μg h−1 mgcat.−1 and a faradaic efficiency of 12.56%.

Funder

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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