Ambient electrochemical N2-to-NH3 conversion catalyzed by TiO2 decorated juncus effusus-derived carbon microtubes

Author:

Chen Haijun12,Liang Jie3,Dong Kai3ORCID,Yue Luchao3,Li Tingshuai3ORCID,Luo Yongsong3,Feng Zhesheng2,Li Na4ORCID,Hamdy Mohamed S.5,Alshehri Abdulmohsen Ali6,Wang Yan2ORCID,Sun Xuping34ORCID,Liu Qian1

Affiliation:

1. Institute for Advanced Study, Chengdu University, Chengdu 610106, Sichuan, China

2. School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu 611731, Sichuan, China

3. Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, Sichuan, China

4. College of Chemistry, Chemical Engineering and Materials Science, Shandong Normal University, Jinan 250014, Shandong, China

5. Catalysis Research Group (CRG), Department of Chemistry, College of Science, King Khalid University, P.O. Box 9004, 61413 Abha, Saudi Arabia

6. Chemistry Department, Faculty of Science, King Abdulaziz University, P.O. Box 80203, Jeddah 21589, Saudi Arabia

Abstract

TiO2 decorated juncus effusus-derived carbon microtubes (TiO2/JE-CMTs) are highly active and stably for electrochemical N2 reduction to NH3, capable of attaining a large NH3 yield of 20.03 μg h−1 mg−1cat. with a high faradaic efficiency of 10.76%.

Funder

National Natural Science Foundation of China

King Khalid University

Publisher

Royal Society of Chemistry (RSC)

Subject

Inorganic Chemistry

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