A trade-off between ligand and strain effects optimizes the oxygen reduction activity of Pt alloys

Author:

Kluge Regina M.1ORCID,Haid Richard W.1,Riss Alexander2ORCID,Bao Yang2,Seufert Knud2,Schmidt Thorsten O.1ORCID,Watzele Sebastian A.1ORCID,Barth Johannes V.2,Allegretti Francesco2ORCID,Auwärter Willi2ORCID,Calle-Vallejo Federico345ORCID,Bandarenka Aliaksandr S.16ORCID

Affiliation:

1. Physik-Department ECS, Technische Universität München, James-Franck-Straße 1, 85748 Garching, Germany

2. Physik-Department E20, Technische Universität München, James-Franck-Straße 1, 85748 Garching, Germany

3. Nano-Bio Spectroscopy Group and European Theoretical Spectroscopy Facility (ETSF), Department of Polymers and Advanced Materials: Physics, Chemistry and Technology, University of the Basque Country UPV/EHU, Avenida Tolosa 72, 20018 San Sebastián, Spain

4. IKERBASQUE, Basque Foundation for Science, Plaza de Euskadi 5, 48009 Bilbao, Spain

5. Department of Materials Science and Chemical Physics & Institute of Theoretical and Computational Chemistry (IQTCUB), University of Barcelona, Martí i Franquès 1, 08028 Barcelona, Spain

6. Catalysis Research Center TUM, Ernst-Otto-Fischer-Straße 1, 85748 Garching, Germany

Abstract

To optimize the performance of catalytic materials, it is paramount to elucidate the dependence of the chemical reactivity on the atomic arrangement of the catalyst surface.

Funder

Deutsche Forschungsgemeinschaft

Generalitat de Catalunya

Horizon 2020

Agencia Estatal de Investigación

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Nuclear Energy and Engineering,Renewable Energy, Sustainability and the Environment,Environmental Chemistry

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