Breaking scaling relations in nitrogen reduction with asymmetrical heterobimetallic FeCo sites to boost ammonia synthesis-Reference-Cited by-同舟云学术

Breaking scaling relations in nitrogen reduction with asymmetrical heterobimetallic FeCo sites to boost ammonia synthesis

Published:2024 Issue:3 Volume:8 Page:851-858
ISSN:2052-1537
Container-title:Materials Chemistry Frontiers
language:en
Short-container-title:Mater. Chem. Front.

Author:

Xu Na¹²,He Yanzheng¹,Wang Mengfan¹^ORCID,Cheng Chen¹,Cheng Qiyang¹,Liu Sisi¹^ORCID,Ji Haoqing¹,Yan Chenglin¹³^ORCID,Rosei Federico²⁴

Affiliation:

1. College of Energy, Soochow University, Suzhou, 215006, China

2. Institut National de la Recherche Scientifique, 1650 Boul. Lionel-Boulet, Varennes, QC J3X1P7, Canada

3. School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China

4. Department of Chemical and Pharmaceutical Sciences, University of Trieste, Via Giorgeri 1, Trieste 34127, Italy

Abstract

Asymmetrical heterobimetallic FeCo dimer sites featuring a polarized surface with multielectron sites enable weakening of the NN bond and maximized activation of N2, contributing to significantly facilitated ambient ammonia synthesis.

Funder

National Natural Science Foundation of China

Science Fund for Distinguished Young Scholars of Jiangsu Province

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,General Materials Science

Link

http://pubs.rsc.org/en/content/articlepdf/2024/QM/D3QM01076G

Reference57 articles.

1. Turning Waste into Wealth: Sustainable Production of High-Value-Added Chemicals from Catalytic Coupling of Carbon Dioxide and Nitrogenous Small Molecules

2. How to explore ambient electrocatalytic nitrogen reduction reliably and insightfully

3. Awakening (220) as One More Active Facet of PtMo Alloy via Single‐Atom Doping to Boost Ammonia Electrooxidation in Direct Ammonia Fuel Cell

4. Distorted spinel ferrite heterostructure triggered by alkaline earth metal substitution facilitates nitrogen localization and electrocatalytic reduction to ammonia

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