Mechanistic study of the competition between carbon dioxide reduction and hydrogen evolution reaction and selectivity tuning <i>via</i> loading single-atom catalysts on graphitic carbon nitride-Reference-Cited by-同舟云学术

Mechanistic study of the competition between carbon dioxide reduction and hydrogen evolution reaction and selectivity tuning via loading single-atom catalysts on graphitic carbon nitride

Published:2024 Issue:34 Volume:16 Page:16015-16025
ISSN:2040-3364
Container-title:Nanoscale
language:en
Short-container-title:Nanoscale

Author:

Foo Joel Jie¹²,Ng Sue-Faye¹²,Xiong Mo³,Ong Wee-Jun¹²⁴⁵⁶^ORCID

Affiliation:

1. School of Energy and Chemical Engineering, Xiamen University Malaysia, Sepang, Selangor Darul Ehsan, 43900, Malaysia

2. Center of Excellence for NaNo Energy & Catalysis Technology (CONNECT), Xiamen University Malaysia, Sepang, Selangor Darul Ehsan, 43900, Malaysia

3. MOE Key Laboratory for Non-Equilibrium Synthesis and Modulation of Condensed Matter, School of Physics, Xi'an Jiaotong University, Xi'an 710049, Shanxi, China

4. State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China

5. Gulei Innovation Institute, Xiamen University, Zhangzhou 363200, China

6. Shenzhen Research Institute of Xiamen University, Shenzhen, 518057, China

Abstract

We computationally screened metal-single-atom catalysts (M-SAC) on carbon nitride for selective CO2 reduction. NiCN significantly lowered the rate-determining potential for CO2 conversion to formic acid via the *OCHO key intermediate.

Funder

State Key Laboratory of Physical Chemistry of Solid Surfaces, Xiamen University

Kementerian Sains, Teknologi dan Inovasi

National Natural Science Foundation of China

Ministry of Higher Education, Malaysia

Basic and Applied Basic Research Foundation of Guangdong Province

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/NR/D4NR01932F

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