Relaxation dynamics in excited helium nanodroplets probed with high resolution, time-resolved photoelectron spectroscopy

Author:

LaForge A. C.1ORCID,Asmussen J. D.2ORCID,Bastian B.2ORCID,Bonanomi M.34,Callegari C.5ORCID,De S.6,Di Fraia M.5ORCID,Gorman L.1,Hartweg S.7ORCID,Krishnan S. R.6ORCID,Kling M. F.891011ORCID,Mishra D.1ORCID,Mandal S.12,Ngai A.7,Pal N.5,Plekan O.5ORCID,Prince K. C.5,Rosenberger P.89ORCID,Aguirre Serrata E.1,Stienkemeier F.7ORCID,Berrah N.1ORCID,Mudrich M.26ORCID

Affiliation:

1. Department of Physics, University of Connecticut, Storrs, Connecticut, 06269, USA

2. Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark

3. Istituto di Fotonica e Nanotecnologie, Consiglio Nazionale delle Ricerche, 20133 Milano, Italy

4. Dipartimento di Fisica Politecnico, 20133 Milano, Italy

5. Elettra-Sincrotrone Trieste S.C.p.A., 34149 Basovizza Trieste, Italy

6. Department of Physics, Indian Institute of Technology-Madras, Chennai 600036, India

7. Institute of Physics, University of Freiburg, 79104 Freiburg im Breisgau, Germany

8. Department of Physics, Ludwig-Maximilians-Universität Munich, 85748 Garching, Germany

9. Max Planck Institute of Quantum Optics, 85748 Garching, Germany

10. SLAC National Accelerator Laboratory, Menlo Park 94025, CA, USA

11. Department of Applied Physics, Stanford University, Stanford 94305, CA, USA

12. Indian Institute of Science Education and Research, Pune 411008, India

Abstract

The ultrafast relaxation dynamics of excited helium nanodroplets were studied using time-resolved photoelectron spectroscopy. We observed an efficient population of triplet atomic states as well as the formation of the first excimer state of He2*.

Funder

U.S. Department of Energy

Deutsche Forschungsgemeinschaft

Max-Planck-Gesellschaft

Carlsbergfondet

Ministry of Education, India

Department of Science and Technology, Ministry of Science and Technology, India

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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