Material design for converting an oxidative-type BiVO4 catalyst into a reductive BiV(S,O)4−x sulfo-oxide catalyst for nitrogen photoreduction to ammonia

Author:

Chen Xiaoyun1ORCID,Zhang Pengkun1,Kuo Dong-Hau2ORCID,Wu Qinhan1,Abdeta Adugna Boke1ORCID,Wu Binghong1,Su Zhengjie1,Chen Longyan1,Zelekew Osman Ahmed3ORCID,Lin Jinguo1

Affiliation:

1. College of Materials Engineering, Fujian Agriculture and Forestry University, Fuzhou 350002, China

2. Department of Materials Science and Engineering, Graduate Institute of Energy and Sustainability Technology, National Taiwan University of Science and Technology, Taipei 10607, Taiwan

3. Department of Materials Science and Engineering, Adama Science and Technology University, Adama, Ethiopia

Abstract

Herein, we demonstrated S2− anion incorporation into BiVO4 for converting an oxidative-type BiVO4 photocatalyst into a reductive-type BiV(S,O)4−x (labeled BiVOS) sulfo-oxide photocatalyst for efficient N2 fixation under an ambient environment.

Funder

National Natural Science Foundation of China

Natural Science Foundation of Fujian Province

Forestry Department of Fujian Province

Fujian Agriculture and Forestry University

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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