Oxygenated P/N co-doped carbon for efficient 2e oxygen reduction to H2O2

Author:

Li Zongge12ORCID,Kumar Anuj3,Liu Nianxi1,Cheng Ming2,Zhao Changkai1,Meng Xiangshe1,Li Huifang4ORCID,Zhang Ying2,Liu Zhiming4ORCID,Zhang Guoxin1ORCID,Sun Xiaoming5ORCID

Affiliation:

1. Department of Energy Storage Technology, Shandong University of Science and Technology, Qingdao 266590, Shandong, China

2. State Key Laboratory of Heavy Oil Processing, China University of Petroleum (East China), Qingdao 266580, Shandong, China

3. Department of Chemistry, GLA University, Mathura 281406, India

4. College of Electromechanical Engineering, Shandong Engineering Laboratory for Preparation and Application of High-performance Carbon-Materials, Qingdao University of Science & Technology, Qingdao 266061, Shandong, China

5. State Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, College of Chemistry, Beijing University of Chemical Technology, Beijing 100029, China

Abstract

Supportive edged P sites that are co-functionalized with O and N atoms yield the best H2O2 yield rate of 698.4 mmol gcat.−1 h−1 and Faradaic efficiency of 87% in a H-type cell.

Funder

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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