Phosphorus-doped Ti3C2Tx MXene nanosheets enabling ambient NH3 synthesis with high current densities

Author:

Qi Yuchuan1,Hou Xianghua1,He Ziying2,He Fan1,Wei Tianran23,Meng Ge12,Hu Huihui3,Liu Qian4,Hu Guangzhi5ORCID,Liu Xijun3ORCID

Affiliation:

1. Key Laboratory of Carbon Materials of Zhejiang Province, College of Chemistry and Materials Engineering, Wenzhou University, Wenzhou 325035, China

2. Guangxi Vocational & Technical Institute of Industry, Nanning 530001, Guangxi, China

3. MOE Key Laboratory of New Processing Technology for Nonferrous Metals and Materials, School of Resources, Environment and Materials, Guangxi University, Nanning, 530004 Guangxi, China

4. Institute for Advanced Study, Chengdu University, Chengdu 610106, Sichuan, China

5. School of Ecology and Environmental Science, Yunnan University, Kunming 650504, China

Abstract

In this work, nitrate reduction to ammonia was achieved using P-doped Ti3C2Tx nanosheets. Impressively, this catalyst showed ampere-level nitrate reduction in a flow cell, implying its potential for sustainable ammonia production.

Funder

National Natural Science Foundation of China

Science Fund for Distinguished Young Scholars of Guangxi Province

Publisher

Royal Society of Chemistry (RSC)

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