Boosting the catalysis of cesium phosphomolybdate encapsulated in hierarchical porous UiO-66 by microenvironment modulation for epoxidation of alkenes

Author:

Hu Dianwen12ORCID,Miao Songsong3,Zhang Pengfei4,Wu Siyuan5,He Yu-Peng12ORCID,Meng Qingwei12ORCID

Affiliation:

1. Ningbo Institute of Dalian University of Technology, Ningbo 315016, China

2. State Key Laboratory of Fine Chemicals, School of Chemical Engineering, Dalian University of Technology, Dalian 116024, China

3. Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China

4. State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Dalian National Laboratory for Clean Energy, Chinese Academy of Sciences, Dalian 116023, China

5. School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai 200237, China

Abstract

CsPM@HP-UiO-66-2CH3 showed preferable catalytic performance in alkene epoxidation reaction among CsPM@HP-UiO-66-X composites, which is mainly attributed to the modulation of the microenvironment surrounding CsPM active sites with a methyl group.

Funder

Dalian University of Technology

Publisher

Royal Society of Chemistry (RSC)

Subject

Inorganic Chemistry

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