Uncovering the influence of the modifier redox potential on CO<sub>2</sub> reduction through combined data-driven machine learning and hypothesis-driven experimentation-Reference-Cited by-同舟云学术

Uncovering the influence of the modifier redox potential on CO₂ reduction through combined data-driven machine learning and hypothesis-driven experimentation

Published:2023 Issue:34 Volume:11 Page:18106-18114
ISSN:2050-7488
Container-title:Journal of Materials Chemistry A
language:en
Short-container-title:J. Mater. Chem. A

Author:

He Xinru¹,Su Yuming¹,Zhu Jieyu¹,Fang Nan¹,Chen YangTao¹,Liu Huichong¹,Zhou Da²,Wang Cheng¹^ORCID

Affiliation:

1. State Key Laboratory of Physical Chemistry of Solid Surfaces, iChem, Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province (IKKEM), College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, P. R. China

2. School of Mathematical Sciences, Xiamen University, Xiamen 361005, China

Abstract

By examining the literature on organic-modified Cu in CO2 electroreduction and conducting tailored experiments, we discovered a link between the reduction potential of the modifier and the selectivity of the resulting products.

Funder

National Natural Science Foundation of China

National Key Research and Development Program of China

Fundamental Research Funds for the Central Universities

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2023/TA/D3TA03115B

Reference43 articles.

1. Opportunities for Electrocatalytic CO₂ Reduction Enabled by Surface Ligands

2. Hydrophobic Copper Interfaces Boost Electroreduction of Carbon Dioxide to Ethylene in Water

3. Tailored catalyst microenvironments for CO2 electroreduction to multicarbon products on copper using bilayer ionomer coatings

4. Hydrogen bonding steers the product selectivity of electrocatalytic CO reduction

5. Reorganization of Interfacial Water by an Amphiphilic Cationic Surfactant Promotes CO2 Reduction

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