Chemoselective, osmium-free, dihydroxylation/oxidative cleavage of heteroaryl isoprenes by a contemporary Malaprade reaction-Reference-Cited by-同舟云学术

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Chemoselective, osmium-free, dihydroxylation/oxidative cleavage of heteroaryl isoprenes by a contemporary Malaprade reaction

Published:2022 Issue:40 Volume:20 Page:7916-7922
ISSN:1477-0520
Container-title:Organic & Biomolecular Chemistry
language:en
Short-container-title:Org. Biomol. Chem.

Author:

Gulledge Zachary Z.¹,Pinson Connor C.¹,Stovall Alexander M.¹,Dzeagu Fortune O.¹,Carrick Jesse D.¹^ORCID

Affiliation:

1. Department of Chemistry, Tennessee Technological University, Cookeville, TN 38505-0001, USA

Abstract

Dihydroxylation/oxidative cleavage of functionalized isoprenes leveraging KMnO4 as a greener alternative to OsO4 chemoselectively affords heteroaryl methyl ketones.

Funder

U.S. Department of Energy

Basic Energy Sciences

Publisher

Royal Society of Chemistry (RSC)

Subject

Organic Chemistry,Physical and Theoretical Chemistry,Biochemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2022/OB/D2OB01643E

Reference24 articles.

1. Synthesis of 1H-Pyrazol-5-yl-pyridin-2-yl-[1,2,4]triazinyl Soft-Lewis Basic Complexants via Metal and Oxidant Free [3 + 2] Dipolar Cycloaddition of Terminal Ethynyl Pyridines with Tosylhydrazides

2. G. A.Olah , Interscience Monographs on Organic Chemistry: Friedel-Crafts Chemistry , Wiley-Interscience , New York, N. Y. , 1973 , p. 581

3. Synthetic Approaches to Polypyridyl Bridging Ligands with Proximal Multidentate Binding Sites

4. Catalytic Asymmetric Dihydroxylation

5. Discovery of a Practical Direct O2-Coupled Wacker Oxidation with Pd[(−)-sparteine]Cl2

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