Identification of non-metal single atomic phosphorus active sites for the CO2 reduction reaction

Author:

Bin Yang Hong1,Xu Cong-Qiao2ORCID,Baskaran Sambath2,Lu Ying-Rui3,Gu Chengding4,Liu Wei5ORCID,Ding Jie1,Zhang Jincheng1,Wang Qilun1ORCID,Chen Wei5,Li Jun26ORCID,Huang Yanqiang7ORCID,Zhang Tao7,Liu Bin1ORCID

Affiliation:

1. Department of Materials Science and Engineering, City University of Hong Kong, Hong Kong SAR 999077, China

2. Department of Chemistry, Southern University of Science and Technology, Shenzhen 518055, China

3. National Synchrotron Radiation Research Center, Hsinchu, 30076, Taiwan

4. School of Materials and Energy, Yunnan University, 650091, China

5. Department of Chemistry, National University of Singapore, 3 Science Drive 3, 117543, Singapore

6. Department of Chemistry and Key Laboratory of Organic Optoelectronics and Molecular Engineering of Ministry of Education, Tsinghua University, Beijing 100084, China

7. Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China

Abstract

Due to intrinsic difference between non-metal atoms and metal atoms, SACs with non-metal centers will also have unique characteristics, which would cause changes in the adsorption configuration of reaction intermediates, thereby regulating the reaction path.

Funder

Guangdong Provincial Key Laboratory Of Catalysis

National Natural Science Foundation of China

Chinese Academy of Sciences

Publisher

Royal Society of Chemistry (RSC)

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