Seed- and solvent-free synthesis of ZSM-5 with tuneable Si/Al ratios for biomass hydrogenation-Reference-Cited by-同舟云学术

Seed- and solvent-free synthesis of ZSM-5 with tuneable Si/Al ratios for biomass hydrogenation

Published:2020 Issue:5 Volume:22 Page:1630-1638
ISSN:1463-9262
Container-title:Green Chemistry
language:en
Short-container-title:Green Chem.

Author:

Zhang Bin¹²³⁴⁵^ORCID,Douthwaite Mark⁶⁷⁸⁹¹⁰,Liu Qiang¹²³⁴⁵,Zhang Chao¹²³⁴⁵^ORCID,Wu Qifan¹²³⁴⁵,Shi Ruhui¹²³⁴⁵,Wu Peixuan¹²³⁴⁵,Liu Ke¹²³⁴⁵,Wang Zhuangqing¹²³⁴⁵,Lin Weiwei¹²³⁴⁵^ORCID,Cheng Haiyang¹²³⁴⁵^ORCID,Ma Ding¹¹¹²¹³¹⁴¹⁵^ORCID,Zhao Fengyu¹²³⁴⁵^ORCID,Hutchings Graham J.⁶⁷⁸⁹¹⁰^ORCID

Affiliation:

1. State Key Laboratory of Electroanalytical Chemistry and Laboratory of Green Chemistry and Process

2. Changchun Institute of Applied Chemistry

3. Chinese Academy of Sciences

4. Changchun 130022

5. China

6. Cardiff Catalysis Institute

7. School of Chemistry

8. Cardiff University

9. Cardiff

10. UK

11. Beijing National Laboratory for Molecular Sciences

12. College of Chemistry and Molecular Engineering and College of Engineering

13. and BIC-ESAT

14. Peking University

15. Beijing 100871

Abstract

Seed- and solvent-free synthesis of MFI zeolites with tuneable Si/Al ratios (18-∞) was achieved. The key role of F⁻ was evidenced that forming 6-coordinated “F–Al–O–Si” species drove the formation of the zeolitic framework during crystallization.

Funder

National Natural Science Foundation of China

National Basic Research Program of China

Youth Innovation Promotion Association of the Chinese Academy of Sciences

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Environmental Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2020/GC/C9GC03622A

Reference51 articles.

1. Shape-selective zeolite catalysis for bioplastics production