Catalytic <i>tert</i>-alkylation of enamides <i>via</i> C–C bond cleavage under photoredox conditions-Reference-Cited by-同舟云学术

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Catalytic tert-alkylation of enamides via C–C bond cleavage under photoredox conditions

Published:2024 Issue:52 Volume:60 Page:6623-6626
ISSN:1359-7345
Container-title:Chemical Communications
language:en
Short-container-title:Chem. Commun.

Author:

Tsuchiya Naoki¹,Oku Ayane¹,Nishikata Takashi¹^ORCID

Affiliation:

1. Graduate School of Science and Engineering, Yamaguchi University, 2-16-1 Tokiwadai, Ube, Yamaguchi, 755-8611, Japan

Abstract

Efficient C–C bond cleavage is recognized as a persistent challenge in the field of synthetic methodology. In this paper, we found that tert-alkylated cyclohexadienones are good tert-alkyl radical donors in the presence of photocatalysts and that olefination with enamides proceeds.

Funder

Yamaguchi University

Japan Science and Technology Corporation

Japan Society for the Promotion of Science

Ministry of the Environment, Government of Japan

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/CC/D4CC01643B

Reference56 articles.

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2. S. Z.Zard , Radical Reactions in Organic Synthesis , Oxford, New York , 2003

3. Encyclopedia of Radicals in Chemistry, Biology and Materials , eds. C. Chatgilialoglu , A. Studer , Wiley-Interscience , 2012 , vol. 2

4. Formation of CC Bonds by Addition of Free Radicals to Alkenes

5. The invention of radical reactions. Part XIX. The synthesis of very hindered quinones

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