Near 100% selectivity for ammonia synthesis at a high current density by promoting nitrate protonation on the copper dispersed todorokite-type manganese oxide-Reference-Cited by-同舟云学术

Near 100% selectivity for ammonia synthesis at a high current density by promoting nitrate protonation on the copper dispersed todorokite-type manganese oxide

Published:2023 Issue:24 Volume:25 Page:10549-10555
ISSN:1463-9262
Container-title:Green Chemistry
language:en
Short-container-title:Green Chem.

Author:

Li Shijia¹^ORCID,Xiao Chuqian¹,Chen Rongzhen¹,Wang Mengyi¹,Ma Yuting¹,Luo Kaiwen¹,Shen Muyao¹,Zhu Yihua¹^ORCID,Li Yuhang¹^ORCID,Li Chunzhong¹²^ORCID

Affiliation:

1. Key Laboratory for Ultrafine Materials of Ministry of Education, Shanghai Engineering Research Center of Hierarchical Nanomaterials, Frontiers Science Center for Materiobiology and Dynamic Chemistry, School of Materials Science and Engineering, East China University of Science & Technology, Shanghai 200237, China

2. School of Chemical Engineering, East China University of Science & Technology, Shanghai 200237, China

Abstract

The Cu-dispersed OMS-1 promotes NO3− protonation to produce ammonia with a Faraday efficiency of ∼100% and production rate of 0.51 mmol h−1 cm−2.

Funder

Science and Technology Commission of Shanghai Municipality

Fundamental Research Funds for the Central Universities

Shanghai Rising-Star Program

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Environmental Chemistry