Bifunctional catalyst MoSx@H-Beta for highly selective conversion of CO2 to C2–6 hydrocarbons

Author:

Zhao Taotao1,Shen Chenyang1,Liu Yuchi1,Liu Gui1,Qian Xiaofeng1,He Qiang1,Mei Feifei1,He Yu1,Guo Xiangke1,Xue Nianhua1,Liu Xi2ORCID,Ding Weiping1ORCID

Affiliation:

1. Key Lab of Mesoscopic Chemistry, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210023, China

2. School of Chemistry and Chemical, In-situ Centre for Physical Sciences, Frontiers Science Centre for Transformative Molecules, Shanghai Jiao Tong University, Shanghai, 200240, P. R. China

Abstract

MoSx clusters encapsulated in channels of H-Beta zeolite constitute a bifunctional catalyst and show excellent catalytic performance for CO2 hydrogenation: CO2 conversion >13%, C2–6 hydrocarbons selectivity >74% and stability >200 h on stream.

Funder

National Science and Technology Major Project

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

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