Mechanism and structure–activity relationship of H2 and CO2 activation at the ZnO/Cu catalyst interface

Author:

Xin Xin12ORCID,Gao Peng123ORCID,Li Shenggang1234ORCID

Affiliation:

1. CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences, 100 Haike Road, Shanghai 201210, China

2. University of Chinese Academy of Sciences, Beijing 100049, China

3. State Key Laboratory of Low Carbon Catalysis and Carbon Dioxide Utilization, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201210, China

4. School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China

Abstract

The ZnO/Cu interface is predicted to promote hydrogen activation and spillover to form interfacial oxygen vacancies, enhancing CO2 reactivity during its hydrogenation.

Funder

National Natural Science Foundation of China

Program of Shanghai Academic Research Leader

Science and Technology Commission of Shanghai Municipality

Publisher

Royal Society of Chemistry (RSC)

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