Non-steady state validation of kinetic models for ethylene epoxidation over silver catalysts-Reference-Cited by-同舟云学术

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Non-steady state validation of kinetic models for ethylene epoxidation over silver catalysts

Published:2024 Issue:13 Volume:14 Page:3596-3608
ISSN:2044-4753
Container-title:Catalysis Science & Technology
language:en
Short-container-title:Catal. Sci. Technol.

Author:

Brandão Lilliana¹^ORCID,Reece Christian¹^ORCID

Affiliation:

1. Rowland Institute at Harvard, Harvard University, Cambridge, Massachusetts 02142, USA

Abstract

A two-site kinetic model for ethylene epoxidation most accurately recreates the selectivity trends observed during transient pressure pulse experiments of ethylene over oxidized silver.

Funder

Rowland Institute at Harvard

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/CY/D4CY00052H

Reference31 articles.

1. AgileIntel Research (ChemIntel360), Market value of ethylene oxide worldwide from 2015 to 2022, with a forecast for 2023 to 2030, https://www.statista.com/statistics/1244434/global-market-value-ethylene-oxide/ , (accessed August 2, 2023)

2. Overview of Selective Oxidation of Ethylene to Ethylene Oxide by Ag Catalysts

3. Construction of a reaction coordinate and a microkinetic model for ethylene epoxidation on silver from DFT calculations and surface science experiments

4. Ethylene Epoxidation on Ag(100), Ag(110), and Ag(111): A Joint Ab Initio and Kinetic Monte Carlo Study and Comparison with Experiments

5. Microkinetic modeling of ethylene oxidation over silver

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