Fluorinated polymer zwitterions on gold nanoparticles: patterned catalyst surfaces guide interfacial transport and electrochemical CO2 reduction

Author:

Luo Qiang1ORCID,Tapia Joseph2ORCID,Zhou Le3,Liu Chung-Hao45ORCID,Liaqat Maham1,Duan Hanyi4ORCID,Yang Zhefei3ORCID,Nieh Mu-Ping46ORCID,Emrick Todd3ORCID,Bai Peng2ORCID,He Jie14ORCID

Affiliation:

1. Department of Chemistry, University of Connecticut, Storrs, CT 06269, USA

2. Department of Chemical Engineering, University of Massachusetts, Amherst, Massachusetts 01003, USA

3. Polymer Science and Engineering Department, Conte Center for Polymer Research University of Massachusetts, Amherst, Massachusetts 01003, USA

4. Polymer Program, Institute of Materials Science, University of Connecticut, Storrs, CT 06269, USA

5. Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA

6. Department of Chemical and Biomolecular Engineering, University of Connecticut, Storrs, CT 06269, USA

Abstract

We report the use of fluorinated polymer zwitterions to build hybrid systems for efficient CO2 electroreduction.

Funder

Division of Chemical, Bioengineering, Environmental, and Transport Systems

U.S. Department of Energy

Basic Energy Sciences

Division of Materials Sciences and Engineering

National Institutes of Health

National Institute of General Medical Sciences

Brookhaven National Laboratory

Office of Science

National Science Foundation

Publisher

Royal Society of Chemistry (RSC)

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