Very strong interaction between FeN4 and titanium carbide for durable 4-electron oxygen reduction reaction suppressing catalyst deactivation by peroxide

Author:

Lee Yeongdae1,Ahn Jang Hyuk1,Jang Haeseong2,Lee Jisu1,Yoon Subhin1,Lee Dong-Gyu1,Kim Min Gyu2ORCID,Lee Jun Hee1,Song Hyun-Kon1ORCID

Affiliation:

1. School of Energy and Chemical Engineering, UNIST, Ulsan 44919, Korea

2. Beamline Research Division, Pohang Accelerator Laboratory (PAL), Pohang 37673, Korea

Abstract

Very strong catalyst–support interaction was realized by supporting FePc with Ti3C2, encouraging biased electron transfer to Fe. 4e ORR activity was improved to suppress peroxide production and therefore to have ORR durability guaranteed.

Funder

National Research Foundation of Korea

Ministry of Trade, Industry and Energy

Ulsan National Institute of Science and Technology

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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