Unconventional direct synthesis of Ni3N/Ni with N-vacancies for efficient and stable hydrogen evolution

Author:

Zhang Doudou1ORCID,Li Haobo2,Riaz Asim3ORCID,Sharma Astha1ORCID,Liang Wensheng1,Wang Yuan4ORCID,Chen Hongjun5,Vora Kaushal3,Yan Di1,Su Zhen4,Tricoli Antonio5ORCID,Zhao Chuan4ORCID,Beck Fiona J.1ORCID,Reuter Karsten26,Catchpole Kylie1,Karuturi Siva13ORCID

Affiliation:

1. School of Engineering, The Australian National University Canberra, ACT 2601, Australia

2. Theoretical Chemistry and Catalysis Research Center, Technische Universität München, Lichtenbergstr. 4, 85747 Garching, Germany

3. Department of Electronic Materials Engineering, Research School of Physics, The Australian National University Canberra, ACT 2601, Australia

4. School of Chemistry, Faculty of Science, The University of New South Wales, Sydney, NSW 2052, Australia

5. Nanotechnology Research Laboratory, Faculty of Engineering, University of Sydney, NSW 2006, Australia

6. Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, 14195 Berlin, Germany

Abstract

Direct synthesis of Ni3N/Ni catalyst enriched with N-vacancies using one-step reactive magnetron sputtering with enhanced performance for the hydrogen evolution reaction in photoelectrochemical cells and electrolysers.

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Nuclear Energy and Engineering,Renewable Energy, Sustainability and the Environment,Environmental Chemistry

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