Synergistic defect- and interfacial-engineering of a Bi2S3-based nanoplate network for high-performance photoelectrochemical solar water splitting

Author:

Wang Ying1,Liu Min2,Hao Shiqiang3,Li Yuan45ORCID,Li Qianqian6,Liu Fangyang1ORCID,Lai Yanqing1,Li Jie1,Wolverton Chris3ORCID,Dravid Vinayak P.3ORCID,Jiang Liangxing1ORCID

Affiliation:

1. School of Metallurgy and Environment, Central South University, Changsha, Hunan 410083, China

2. School of Physics and Electronics, Central South University, Changsha, Hunan 410083, China

3. Northwestern University Atomic and Nanoscale Characterization Experimental (NUANCE) Centre, Department of Materials Science and Engineering, Northwestern University, Evanston, Illinois 60208, USA

4. State Key Laboratory of Material Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan, Hubei 430074, China

5. Shenzhen Huazhong University of Science and Technology Research Institute, Shenzhen 518057, China

6. Materials Genome Institute, Shanghai University, Shanghai 200444, China

Abstract

Successful modulation of photoelectrochemical performance of Bi2S3 nanowalls was achieved by a synergistic defect- and interface-engineering strategy, which renders significantly improved charge separation and transfer efficiency in water splitting.

Funder

National Natural Science Foundation of China

Natural Science Foundation of Hunan Province

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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