Environmentally sustainable lithium-ion battery cathode binders based on cellulose nanocrystals

Author:

Huang Xingkang12ORCID,You Haoyang3ORCID,Yan Xiaoli4,Borkiewicz Olaf J.5,Wiaderek Kamila M.5,Hui Janan6,Hersam Mark C.678ORCID,Chaudhuri Santanu49,Rowan Stuart J.123ORCID,Chen Junhong12ORCID

Affiliation:

1. Pritzker School of Molecular Engineering, The University of Chicago, 5640 S. Ellis Ave, Chicago, IL, 60637, USA

2. Chemical Sciences and Engineering Division, Physical Sciences and Engineering Directorate, Argonne National Laboratory, Lemont, Illinois 60439, USA

3. Department of Chemistry, The University of Chicago, Chicago, IL, 60637, USA

4. Department of Civil, Materials, and Environmental Engineering, University of Illinois, Chicago, Illinois, 60439, USA

5. X-ray Science Division, Advanced Photon Source, Argonne National Laboratory, Lemont, IL 60439, USA

6. Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208, USA

7. Department of Chemistry, Northwestern University, Evanston, IL 60208, USA

8. Department of Electrical and Computer Engineering, Northwestern University, Evanston, IL 60208, USA

9. Applied Materials Division, Advanced Energy Technologies Directorate, Argonne National Laboratory, Lemont, IL, 60439, USA

Abstract

Carboxylic acid functionalized cellulose nanocrystals have been obtained from biomass and evaluated as aqueous, environmentally sustainable alternatives to conventional polyvinylidene difluoride binders for cathodes of lithium-ion batteries.

Funder

Basic Energy Sciences

Directorate for Engineering

National Science Foundation

Publisher

Royal Society of Chemistry (RSC)

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