Biomass-derived oxygen-doped hollow carbon microtubes for electrocatalytic N2-to-NH3 fixation under ambient conditions-Reference-Cited by-同舟云学术

Biomass-derived oxygen-doped hollow carbon microtubes for electrocatalytic N2-to-NH3 fixation under ambient conditions

Published:2019 Issue:18 Volume:55 Page:2684-2687
ISSN:1359-7345
Container-title:Chemical Communications
language:en
Short-container-title:Chem. Commun.

Author:

Wu Tengteng¹²³⁴⁵,Li Peipei¹²³⁴⁵,Wang Huanbo⁶⁷⁸⁵,Zhao Runbo⁹¹⁰¹¹⁵^ORCID,Zhou Qiang¹²⁷¹³⁵,Kong Wenhan⁶⁷⁸⁵,Liu Meiling¹²³⁴⁵^ORCID,Zhang Youyu¹²³⁴⁵^ORCID,Sun Xuping⁶⁷⁸⁵^ORCID,Gong Feng (Frank)¹²⁷¹³⁵^ORCID

Affiliation:

1. Key Laboratory of Chemical Biology and Traditional Chinese Medicine Research (Ministry of Education)

2. College of Chemistry and Chemical Engineering

3. Hunan Normal University

4. Changsha 410081

5. China

6. Institute of Fundamental and Frontier Sciences

7. University of Electronic Science and Technology of China

8. Chengdu 610054

9. School of Environment and Resource

10. Southwest University of Science and Technology

11. Mianyang 621010

12. School of Materials and Energy

13. Chengdu 611731

Abstract

Oxygen-doped hollow carbon microtubes electrocatalyze the N₂-to-NH₃ fixation with a faradaic efficiency of 9.1% and a NH₃ yield rate of 25.12 μg h⁻¹ mg_cat.⁻¹ at −0.80 V and −0.85 V vs. RHE, respectively.

Funder

National Natural Science Foundation of China

Education Department of Hunan Province

Hunan Provincial Science and Technology Department

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,Metals and Alloys,Surfaces, Coatings and Films,General Chemistry,Ceramics and Composites,Electronic, Optical and Magnetic Materials,Catalysis

Link

http://pubs.rsc.org/en/content/articlepdf/2019/CC/C8CC09867K

Reference39 articles.

1. Catalytic Synthesis of Ammonia—A “Never-Ending Story”?

2. T. Vegge , R. Z.Sørensen , A.Klerke , J. S.Hummelshøj , T.Johannessen , J. K.Nørskov and C. H.Christensen , Indirect Hydrogen Storage in Metal Ammines, Solid-State Hydrogen Storage , 2008 , pp. 533–564

3. J. R. Jennings , Catalytic ammonia synthesis: fundamentals and practice , Spring Science & Business Media , 1991

4. Recent progress towards the electrosynthesis of ammonia from sustainable resources

5. Progress in the Electrochemical Synthesis of Ammonia

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